假电容
超级电容器
氧化还原
阴极
水溶液
储能
材料科学
化学
氮气
化学工程
无机化学
碳纤维
电容
电极
有机化学
物理化学
复合材料
复合数
功率(物理)
工程类
物理
量子力学
作者
Xin Shi,Haozhe Zhang,Siqi Zeng,Jin Wang,Xianshuo Cao,Xiaoqing Liu,Xihong Lu
出处
期刊:ACS materials letters
[American Chemical Society]
日期:2021-08-02
卷期号:3 (9): 1291-1299
被引量:63
标识
DOI:10.1021/acsmaterialslett.1c00325
摘要
The development of high-performance, low-cost carbon cathodes is desperately desired but remains challenging for further widespread application of aqueous Zn-ion hybrid supercapacitors (ZHSCs). Herein, we propose nitrogen-doped carbon materials derived from inexpensive industrial byproducts, pitch, as advanced ZHSCs cathodes. The nitrogen dopants significantly enhance the conductivity of pitch-derived carbon while the electrochemically active pyrrolic nitrogen substantially accelerates the reaction kinetics for energy storage and yields more pseudocapacitance via nitrogen redox mechanism. Consequently, the as-designed cathode shows satisfactory Zn ion storage ability as well as distinct anti self-discharge ability resulting. When assembled as a ZHSC device, the supercapacitor delivers a high capacity of 136.2 mA h g–1, excellent rate performance (50.8% capacity retention from 0.3 A g–1 to 15 A g–1) and satisfactory anti self-discharge ability (only 4.6% capacity loss after 24 h rest). This finding highlights the potential high-value utilization of industry byproducts and provides insight for understanding nitrogen redox chemistry in aqueous energy storage.
科研通智能强力驱动
Strongly Powered by AbleSci AI