High frequency acoustic microscopy imaging of pellet cladding interface in nuclear fuel rods

颗粒 包层(金属加工) 材料科学 弹丸 核燃料 陶瓷 辐照 锆合金 复合材料 扫描电子显微镜 光学显微镜 声学显微镜 核工程 显微镜 光学 显微镜 核物理学 工程类 物理 病理 替代医学 医学 合金
作者
Hajar Saikouk,Didier Laux,Brigitte Lacroix,Eric Frederici,Emmanuel Le Clézio,Gilles Despaux
出处
期刊:Nuclear Engineering and Design [Elsevier]
卷期号:417: 112844-112844
标识
DOI:10.1016/j.nucengdes.2023.112844
摘要

In Pressurized Water Reactors (PWRs), fuel rods play a crucial role in generating nuclear energy. These rods consist of ceramic pellets, such as UO2 or (U,Pu)O2, enclosed in a zircaloy cladding tube, leaving an initial gap between the pellets and the cladding. As the reactor operates and the fuel undergoes irradiation, both the ceramic pellets and the zircaloy cladding experience transformations, causing the gap between them to gradually close. This phenomenon has a significant impact on the thermomechanical behavior of the fuel rod. Understanding the nature of the bonding that occurs during irradiation is essential for ensuring the safe and efficient operation of the reactor. To investigate the evolution of the contact state between the fuel pellets and the cladding during irradiation, a detailed analysis of the pellet-cladding interface after irradiation is necessary. However, traditional examination methods might be destructive or incapable of providing the desired level of precision and resolution. The Institute of Electronic and Systems at the University of Montpellier (IES – UMR CNRS 5214), in collaboration with the Alternative Energies and Atomic Energy Commission (CEA) and Electricité de France (EDF), has developed a specialized high-frequency acoustic microscope for imaging and non-destructively inspecting the pellet/cladding interface. The design of the acoustic microscope takes into account the complexity of the fuel rod's structure and the challenges associated with imaging the pellet/cladding interface by utilizing high-frequency ultrasound. In this paper, we present the ability of this acoustic microscope to acquire 2D images with controlled displacements of the sample rod along both its axial and circumferential directions thanks to a card with a high sampling frequency reaching 2 GHz. This capability is crucial because the geometrical, chemical, and mechanical properties of the fuel pellet-cladding contact are not uniform in these directions. By obtaining detailed acoustic images, we can identify specific regions where the fuel pellets and the cladding were in contact during irradiation. In this research, a resolution study is carried out to validate the microscope's ability to investigate the fuel rod and achieve the desired resolutions. Testing on real samples requires a specific configuration of the microscope, which must be adapted to the irradiation conditions. This is why, before proceeding to this stage, it is necessary to carry out tests on representative samples to validate the achievement of the desired resolution. So we’re also presenting the first acoustic images obtained on the zircaloy alloy claddings.
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