光催化
材料科学
异质结
正交晶系
单斜晶系
兴奋剂
铋
氧气
钙钛矿(结构)
化学工程
晶体结构
光电子学
化学
催化作用
结晶学
有机化学
工程类
冶金
作者
Li Lv,Lei Lin,Qi‐Wen Chen,Chang‐Ling Yin,Huiqing Fan,Jianping Zhou
标识
DOI:10.1016/j.apcatb.2023.123464
摘要
Monoclinic phase La2Ti2O7 and orthorhombic phase Bi4Ti3O12 with layered crystal structure constructed by the perovskite slab were widely used in photocatalysis. Their electronic structures are the most crucial factor in high photocatalytic activity. Bi-doped La2Ti2O7 gradually converts to La-doped Bi4Ti3O12 with the incorporation of bismuth ions, and the two phases build an S-scheme heterojunction. More oxygen vacancies were introduced into the S-scheme heterojunction after heat treatment in a nitrogen atmosphere. The 0.1BTO/LTO-OV sample exhibits the largest NO removal efficiency of 52% and only 5.6 ppb NO2 intermediate generation. The improved NO removal efficiency was ascribed to the synergistic effect of oxygen vacancies, doping and heterojunction, providing a new insight into the photocatalytic NO removal. The photocatalytic mechanism was eventually proposed on the basis of trapping experiments.
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