Magnetism and spin dynamics of the S = 32 frustrated trillium lattice compound K2CrTi(

The subtle interplay between competing degrees of freedom offers an ideal route for the experimental realization of emergent quantum and topological phenomena with exotic quasiparticle excitations in three-dimensional noncentrosymmetric frustrated magnets on a trillium lattice. Here, the authors demonstrate the coexistence of competing magnetic states and short-range spin correlations well above the magnetic phase transition in a frustrated double trillium lattice comprised of Cr${}^{3+}$ ions decorated on a three-dimensional chiral network of corner-shared equilateral triangular motifs.