A high strength and flexible multilayered thin film laser induced graphene heater for thermal applications

Increasing demand for wearable sensors and heating elements has occurred recently. Herein, graphene has been observed as a biocompatible, cost effective, and multidimensional material catering to both sensing and heating applications. However, it still lacks essential features such as high temperature performance with low power usage, high strength, and robustness of thin films in tough environments such as heating elements in thermal socks. Hence, in this paper, we demonstrated laser induced graphene (LIG) as a suitable candidate for wearable thermal applications. LIG heaters were fabricated using a cost effective and environmentally friendly technique based on photothermal ablation of polyimide substrate using a 50 W CO2 laser. The heat flux of LIG heater was improved by stacking multiple films while their electrical connections are made in parallel. Upon joule heating, the heaters had excellent electrothermal performance, fast and stable response, achieving temperature of 195 °C using a relatively low DC voltage of 10 V. Most importantly, they showed good durability after bending, washing and repeated heating and cooling cycles. Due to these advantages, the LIG-based thin film heaters have potential as reliable and low-cost heating elements for variety of tough applications such as defrosting and wearable thermal pads.