超导电性
钪
凝聚态物理
临界场
相干长度
软化
材料科学
物理
量子力学
冶金
作者
Kui Wang,Yao Sun,Mi Zhou,Hanyu Liu,Guangchen Ma,Hongbo Wang,Guangtao Liu,Yanming Ma
标识
DOI:10.1103/physrevresearch.5.043248
摘要
The pursuit of elemental superconductors with high critical temperature $({T}_{c})$ holds immense scientific significance due to their relatively simple material composition, which not only aids in understanding the mechanisms of superconductivity but also facilitates further exploration of high-temperature superconductors in compound materials. Here, we report experimental findings of superconductivity for scandium (Sc) in the pressure range of 64 GPa to 261 GPa. As a result, the highest ${T}_{c}$ of 37.6 K observed in Sc-V phase at 243 GPa sets the current record among all elements. An estimate based on the Ginzburg-Landau model gives a zero-temperature upper critical magnetic field of 21.3 T with a coherence length of 39.3 \AA{}. Current-voltage measurements show that the zero-temperature critical current and its density can reach 0.146 A and 70 A ${\mathrm{mm}}^{\ensuremath{-}2}$ of Sc-IV at 198 GPa, and 0.116 A and 50 A ${\mathrm{mm}}^{\ensuremath{-}2}$ of Sc-V at 250 GPa, respectively. Further theoretical calculations show that pressure-induced phonon softening plays a key role in increasing ${T}_{c}$ upon compression. Our current findings shed light on the understanding of high superconductivity in simple elements and provide insight into exploring high-${T}_{c}$ elemental superconductors and Sc-based superconductors.
科研通智能强力驱动
Strongly Powered by AbleSci AI