Employment of relaxation times distribution with improved elastic net regularization for advanced impedance data analysis of a lithium-ion battery

电阻抗 正规化(语言学) 阻抗参数 计算机科学 介电谱 等效电路 锂离子电池 极化(电化学) 生物系统 算法 电子工程 材料科学 电池(电) 化学 电压 电化学 电气工程 电极 工程类 物理 人工智能 热力学 物理化学 功率(物理) 生物
作者
Roland Kobla Tagayi,Salah Eddine Ezahedi,Jaeyeong Kim,Jonghoon Kim
出处
期刊:Journal of energy storage [Elsevier BV]
卷期号:70: 107970-107970 被引量:7
标识
DOI:10.1016/j.est.2023.107970
摘要

Electrochemical impedance spectroscopy (EIS) is a familiar conventional approach that has been widely applied to analyze electrochemical systems, such as batteries and fuel cells, to determine the polarization resistances of their electrodes. An improved method that can effectively interpret EIS spectra with high resolution and provide close knowledge of the time features of the electrochemical system being considered is the distribution of relaxation times (DRT). However, estimating and attaining DRT is a challenging issue that involves solutions being obtained by employing regularization techniques. This study proposed an improved elastic net (IEN) regularization with an adaptive elastic net penalty, wherein adaptive weight matrices were incorporated into the elastic net penalty. The proposed technique was first validated on standard artificial experimental elements: RC circuit, fractal-RC (FRC) circuit, ZARC element, and Gerischer element, each with a known analytical DRT. The results showed that the proposed method exhibited better estimation accuracy in obtaining the exact known DRTs and resistances, and lower mean square errors (MSEs) when compared with the conventional elastic net (EN) regularization method. Furthermore, the proposed method was applied to the EIS data of real lithium-ion batteries with different state-of-charge (SOC) and temperatures, where the obtained DRTs provided an intuitive analysis of the processes within the battery. The proposed model can accurately estimate various time characterizations and identify their processes. Besides the DRTtool results are correspondingly similar to this study's results showing the effectiveness of the proposed approach when compared. However, the limitations and weaknesses of the proposed approach were recognized and reported in this study. Moreover, the proposed approach can be further extended, improved, and employed for advanced EIS techniques and multidimensional EIS data analyses.
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