MXenes公司
材料科学
纳米技术
电池(电)
表面改性
阳极
储能
异质结
电极
化学工程
功率(物理)
光电子学
化学
物理化学
工程类
物理
量子力学
作者
Chao Zheng,Yu Yao,Xianhong Rui,Yuezhan Feng,Dan Yang,Hongge Pan,Yan Yu
标识
DOI:10.1002/adma.202204988
摘要
Abstract MXenes are seen as an exceptional candidate to reshape the future of energy with their viable surface chemistry, ultrathin 2D structure, and excellent electronic conductivity. The extensive research efforts bring about rapid expansion of the MXene families with enriched functionalities, which significantly boost performance of the existing energy‐storage devices. In this review, the strategies that are developed to functionalize the MXene‐based materials, including tailoring their microstructure by ions/molecules/polymers‐initiated interaction or self‐assembly, surface/interface engineering with dopants or functional groups, constructing heterostructures from MXenes with various materials, and transforming them into a series of derivatives inheriting the merits of the MXene precursors are highlighted. Their applications in emerging battery technologies are demonstrated and discussed. With delicate functionalization and structural engineering, MXene‐based electrode materials exhibit improved specific capacity and rate capability, and their presence further suppresses and even eliminates dendrite formation on the metal anodes, which lengthens the lifespan of the rechargeable batteries. Meanwhile, MXenes serve as additives for electrolytes, separators, and current collectors. Finally, some future directions worth of exploration to address the remaining challenging issues of MXene‐based materials and achieve the next‐generation high‐power and low‐cost rechargeable batteries are proposed.
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