等离子体子
手性(物理)
圆二色性
超材料
束缚态
对称性破坏
物理
对称(几何)
纳米光子学
凝聚态物理
量子力学
光学
自发对称破缺
几何学
结晶学
化学
显式对称破缺
数学
作者
Hanan Ali,Simone Zanotti,Giovanni Pellegrini,Emilija Petronijevic,Lucio Claudio Andreani
标识
DOI:10.1021/acsaom.4c00097
摘要
Achieving a strong and robust chiral response in plasmonic metasurfaces is among the key goals of current nanophotonic research. In this work, we theoretically show that the circular dichroism (CD) of a metal metasurface can be maximized by exploiting the concept of a bound state in a continuum (BIC) with symmetry breaking. We consider a gold metasurface with a deformation of circular holes into oval holes. The chiral response at small values of the angle of incidence is dominated by a quasi-BIC, with nearly maximal values of the absorption CD that are almost independent of the deformation. A strong CD in emission is also demonstrated. Symmetry analysis and mode profiles show that the extrinsically chiral response does indeed follow from a symmetry-broken BIC and is associated with a strong enhancement of the local electrical field. The concept of a plasmonic BIC with symmetry breaking provides a robust pathway to increase the chiral response in metal metasurfaces and opens research opportunities in chiral plasmonics that combine narrow resonances with local field enhancement.
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