材料科学
钙钛矿(结构)
发光二极管
光致发光
光电子学
钝化
纳米复合材料
纳米-
等离子体子
表面等离子共振
量子效率
量子点
发光
纳米晶
光子学
纳米颗粒
纳米技术
化学工程
图层(电子)
复合材料
工程类
作者
Ching‐Ho Tien,Hui-Hsuan Tsai,Lung-Chien Chen
标识
DOI:10.1016/j.jmrt.2022.06.109
摘要
Perovskite quantum dots (PeQDs) have a wide range of potential applications in novel displays and solid-state lighting due to their excellent optoelectronic properties. However, insulating ligands around PeQDs can impair the performance of optoelectronic devices. This study proposes a surface ligand passivation of air-synthesized PeQDs modified by incorporation of didodecyl dimethyl ammonium bromide (DDAB), and addition of gold nanoparticles (AuNPs) to induce localized surface plasmon resonance (LSPR) to enhance the photonic characteristics and stability for plasmonic nano-Au:CsPbBr3 perovskite nanocomposite (PeNC), and successfully improved the light-emitting diodes (LEDs) characteristics. The photoluminescence intensity of the nano-Au:CsPbBr3 PeNC film was found to be 1.8-fold higher than that of the pure CsPbBr3 PeQDs film without DDAB. Compare with the pristine PeQD-LEDs without DDAB, the nano-Au:CsPbBr3 PeNC-LEDs thus fabricated exhibit a bright luminance of 6002 cd m−2, corresponding to a 5.4-fold improvement in external quantum efficiency (EQE), whose the device enhancement was attributed to the plasmonic effect of Au NPs.
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