激光阈值
连贯性(哲学赌博策略)
随机激光器
材料科学
激光器
光学
钙钛矿(结构)
光电子学
物理
量子力学
化学
结晶学
作者
Colton Fruhling,Kang Wang,Sarah N. Chowdhury,Xiaohui Xu,Jeffrey Simon,Alexander V. Kildishev,Letian Dou,Xiangeng Meng,Alexandra Boltasseva,Vladimir M. Shalaev
标识
DOI:10.1002/lpor.202200314
摘要
Abstract Quasi‐2D lead halide perovskites have garnered increasing interest as lasing gain media. Relatively simple fabrication, high refractive index, and unique quantum well structure encourage their use in traditional cavity lasers and cavity‐free systems called random lasers (RLs). Despite tremendous advances reported thus far, coherent random lasing in quasi‐2D perovskite subwavelength films has not been reported. Consequently, coherent optical feedback mechanisms in quasi‐2D perovskite systems are still unexplored. Here, this work reports the observation of coherent random lasing in subwavelength quasi‐2D perovskite films. Statistical analysis of spectral measurements reveals Lévy‐like intensity fluctuations, replica symmetry breaking confirms random lasing, and the coherent modes are studied with spectral and spatial correlation techniques. The observed coherent lasing modes are found to be extended states that arise from the random crystal grain structure during fabrication and span the entire pump volume. These modes out‐compete diffusive lasing due to their coherence.
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