Wetting of bio-rejuvenator nanodroplets on bitumen: A molecular dynamics investigation

润湿 接触角 沥青 磁滞 润湿转变 分子动力学 化学物理 材料科学 化学 复合材料 计算化学 凝聚态物理 物理
作者
Haiqin Xu,Yingxue Zou,Gordon Airey,Haopeng Wang,Hanyu Zhang,Shaopeng Wu,Anqi Chen
出处
期刊:Journal of Cleaner Production [Elsevier BV]
卷期号:444: 141140-141140 被引量:26
标识
DOI:10.1016/j.jclepro.2024.141140
摘要

Wetting is the first step during the mix process between rejuvenator and bitumen, which is important for mix efficiency and performance recovery. The wetting of bio-rejuvenator nanodroplets on bitumen was investigated by molecular dynamics (MD) simulations in this research. The bitumen molecule model and bio-rejuvenator nanodroplets were firstly built, then bio-rejuvenator nanodroplets/bitumen interface wetting model were assembled and constructed. Different simulated temperatures were applied to reach equilibrium in the wetting process. Dynamic wetting phenomenon, contact angle of nanodroplets, dynamic movement of nanodroplets, interaction between nanodroplets and bitumen, and hysteresis of contact angle were characterized respectively. The results show that the bio-rejuvenator nanodroplets will first approach the bitumen quickly, and then slow down to an equilibrium state in the wetting process, which delayed 1 ns with energy equilibrium independently. Its contact angle would decrease crossing 90° with time, the equilibrium contact angle of which varies linearly with simulated temperature. The time of nanodroplets reaching partial wetting state decreased with the increments of temperature, but complete wetting state was hard to reach even if the temperature was 433 K. During the nanodroplets movement, contact linear velocity of precursor film and cosine of contact angle was linearly related after nanodroplets and bitumen had caught each other. It was also found that the increasing mix degree was supported by the combination of wetting and infiltration before 373 K and by wetting mainly after 373 K. Finally, the application of external force on bio-rejuvenator nanodroplets will cause hysteresis phenomenon and it can be weakened by higher temperature.
最长约 10秒,即可获得该文献文件

科研通智能强力驱动
Strongly Powered by AbleSci AI
更新
PDF的下载单位、IP信息已删除 (2025-6-4)

科研通是完全免费的文献互助平台,具备全网最快的应助速度,最高的求助完成率。 对每一个文献求助,科研通都将尽心尽力,给求助人一个满意的交代。
实时播报
刚刚
1秒前
韭菜盒子发布了新的文献求助10
3秒前
潘特发布了新的文献求助10
6秒前
乌滴子完成签到,获得积分10
7秒前
量子星尘发布了新的文献求助10
8秒前
善学以致用应助韭菜盒子采纳,获得10
8秒前
jiaaniu完成签到 ,获得积分10
10秒前
清脆靳完成签到,获得积分10
11秒前
cp3xzh完成签到,获得积分10
11秒前
tian发布了新的文献求助10
13秒前
tian发布了新的文献求助10
13秒前
明理宛秋完成签到 ,获得积分10
14秒前
S月小小完成签到,获得积分10
18秒前
斯文的慕儿完成签到 ,获得积分10
25秒前
keen完成签到 ,获得积分10
25秒前
韭菜盒子完成签到,获得积分20
26秒前
潘特完成签到,获得积分10
27秒前
小彭友完成签到,获得积分10
38秒前
39秒前
josie完成签到 ,获得积分10
43秒前
llll完成签到 ,获得积分10
43秒前
量子星尘发布了新的文献求助10
43秒前
韭菜发布了新的文献求助10
43秒前
外向的斑马完成签到 ,获得积分10
44秒前
村长热爱美丽完成签到 ,获得积分10
46秒前
尹尹关注了科研通微信公众号
48秒前
呆呆完成签到 ,获得积分10
49秒前
xianyaoz完成签到 ,获得积分0
56秒前
杨远杰完成签到,获得积分10
57秒前
蓝桉完成签到 ,获得积分10
57秒前
JuliaWang完成签到 ,获得积分10
1分钟前
无限的含羞草完成签到,获得积分10
1分钟前
八二力完成签到 ,获得积分10
1分钟前
韭菜发布了新的文献求助10
1分钟前
情怀应助科研通管家采纳,获得30
1分钟前
water应助科研通管家采纳,获得10
1分钟前
JamesPei应助科研通管家采纳,获得10
1分钟前
2012csc完成签到 ,获得积分0
1分钟前
风清扬应助韭菜采纳,获得10
1分钟前
高分求助中
【提示信息,请勿应助】关于scihub 10000
Les Mantodea de Guyane: Insecta, Polyneoptera [The Mantids of French Guiana] 3000
徐淮辽南地区新元古代叠层石及生物地层 3000
The Mother of All Tableaux: Order, Equivalence, and Geometry in the Large-scale Structure of Optimality Theory 3000
Handbook of Industrial Diamonds.Vol2 1100
Global Eyelash Assessment scale (GEA) 1000
Picture Books with Same-sex Parented Families: Unintentional Censorship 550
热门求助领域 (近24小时)
化学 材料科学 医学 生物 工程类 有机化学 生物化学 物理 内科学 纳米技术 计算机科学 化学工程 复合材料 遗传学 基因 物理化学 催化作用 冶金 细胞生物学 免疫学
热门帖子
关注 科研通微信公众号,转发送积分 4038112
求助须知:如何正确求助?哪些是违规求助? 3575788
关于积分的说明 11373801
捐赠科研通 3305604
什么是DOI,文献DOI怎么找? 1819255
邀请新用户注册赠送积分活动 892655
科研通“疑难数据库(出版商)”最低求助积分说明 815022