环境科学
大气科学
微粒
北京
气溶胶
空气污染
气象学
行星边界层
污染
作者
Zhihao Song,Bin Chen,Jianping Huang
标识
DOI:10.1016/j.envpol.2022.118826
摘要
PM 2.5 (fine particulate matter with aerodynamics diameter <2.5 μm) is the most important component of air pollutants, and has a significant impact on the atmospheric environment and human health. Using satellite remote sensing aerosol optical depth (AOD) to explore the hourly ground PM 2.5 distribution is very helpful for PM 2.5 pollution control. In this study, Himawari-8 AOD, meteorological factors, geographic information, and a new deep forest model were used to construct an AOD-PM 2.5 estimation model in China. Hourly cross-validation results indicated that estimated PM 2.5 values were consistent with the site observation values, with an R 2 range of 0.82–0.91 and root mean square error (RMSE) of 8.79–14.72 μg/m³, among which the model performance reached the optimum value between 13:00 and 15:00 Beijing time (R 2 > 0.9). Analysis of the correlation coefficient between important features and PM 2.5 showed that the model performance was related to AOD and affected by meteorological factors, particularly the boundary layer height. Deep forest can detect diurnal variations in pollutant concentrations, which were higher in the morning, peaked at 10:00–11:00, and then began to decline. High-resolution PM 2.5 concentrations derived from the deep forest model revealed that some cities in China are seriously polluted, such as Xi ‘an, Wuhan, and Chengdu. Our model can also capture the direction of PM 2.5 , which conforms to the wind field. The results indicated that due to the combined effect of wind and mountains, some areas in China experience PM 2.5 pollution accumulation during spring and winter. We need to be vigilant because these areas with high PM 2.5 concentrations typically occur near cities. • The deep forest model effectively captured the hourly PM 2.5 , with R 2 of 0.82–0.91. • Meteorological factors significantly affected the Deep Forest model performance. • Estimated PM 2.5 reflected the pollution condition in city-level areas well. • Seasonal distribution of heavy pollution was related to the wind field and terrain.
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