甲烷
大气甲烷
水槽(地理)
环境科学
大气科学
湿地
甲烷排放
温室气体
氮氧化物
臭氧
一氧化二氮
对流层臭氧
对流层
环境化学
化学
气象学
生态学
海洋学
地质学
地理
有机化学
燃烧
生物
地图学
作者
Shushi Peng,Xin Lin,Rona L Thompson,Yi Xi,Gang Liu,Didier Hauglustaine,Xin Lan,Benjamin Poulter,Michel Ramonet,Marielle Saunois,Yulong Yin,Zhen Zhang,Bo Zheng,Philippe Ciais
出处
期刊:Nature
[Springer Nature]
日期:2022-12-01
卷期号:612 (7940): 477-482
被引量:6
标识
DOI:10.1038/s41586-022-05447-w
摘要
Atmospheric methane growth reached an exceptionally high rate of 15.1 ± 0.4 parts per billion per year in 2020 despite a probable decrease in anthropogenic methane emissions during COVID-19 lockdowns1. Here we quantify changes in methane sources and in its atmospheric sink in 2020 compared with 2019. We find that, globally, total anthropogenic emissions decreased by 1.2 ± 0.1 teragrams of methane per year (Tg CH4 yr-1), fire emissions decreased by 6.5 ± 0.1 Tg CH4 yr-1 and wetland emissions increased by 6.0 ± 2.3 Tg CH4 yr-1. Tropospheric OH concentration decreased by 1.6 ± 0.2 per cent relative to 2019, mainly as a result of lower anthropogenic nitrogen oxide (NOx) emissions and associated lower free tropospheric ozone during pandemic lockdowns2. From atmospheric inversions, we also infer that global net emissions increased by 6.9 ± 2.1 Tg CH4 yr-1 in 2020 relative to 2019, and global methane removal from reaction with OH decreased by 7.5 ± 0.8 Tg CH4 yr-1. Therefore, we attribute the methane growth rate anomaly in 2020 relative to 2019 to lower OH sink (53 ± 10 per cent) and higher natural emissions (47 ± 16 per cent), mostly from wetlands. In line with previous findings3,4, our results imply that wetland methane emissions are sensitive to a warmer and wetter climate and could act as a positive feedback mechanism in the future. Our study also suggests that nitrogen oxide emission trends need to be taken into account when implementing the global anthropogenic methane emissions reduction pledge5.
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