光催化
异质结
材料科学
煅烧
制氢
化学工程
复合数
氢
辐照
可见光谱
纳米技术
催化作用
光电子学
化学
有机化学
复合材料
物理
核物理学
工程类
作者
Xue Jiang,Fan Dong,Xintong Yao,Ziyou Dong,Xinyu Li,Wei Wang,Junchang Liu,Dafeng Zhang,Hengshuai Li,Xipeng Pu,Peiqing Cai
标识
DOI:10.1016/j.jcis.2023.03.055
摘要
The construction of a p-n heterojunction structure is considered to be an effective method to improve the separation of electron-hole pairs in photocatalysts. A series of ZnIn2S4/CoFe2O4 (ZIS/CFO) photocatalysts with p-n heterojunctions were prepared via a method involving ultrasonication and calcination. The synthesized photocatalysts were tested and analyzed via various testing techniques, and their hydrogen evolution rates were evaluated. Compared with pure ZIS, ZIS/CFO with different mass ratios of CFO to ZIS showed improved photocatalytic hydrogen production performance, and the optimal photoactivity showed a nearly 12-fold increase, which can be attributed to the formation of p-n junctions and the formed internal electric field, accelerating the separation of electron-hole pairs and effectively improving the photocatalytic hydrogen evolution rate. The excellent stability of the ZIS/CFO composite was proven by three cycle experiments. In addition, the ZIS/CFO composite also possessed excellent magnetic properties to realize facial magnetic recoverability. This work paves the way for the design and preparation of magnetically recoverable p-n heterojunction photocatalysts.
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