脱氢
钌
甲醇
甲酸
催化作用
化学
氢
级联
水溶液
无机化学
光化学
有机化学
色谱法
作者
Anastasiya Agapova,Henrik Junge,Matthias Beller
标识
DOI:10.1002/chem.201900966
摘要
Abstract A novel state‐of‐the‐art bicatalytic system for hydrogen generation from aqueous methanol at low temperature and base concentration is described. Applying two molecularly defined ruthenium complexes A and B3 for methanol dehydrogenation at the same time under the same conditions, a synergistic effect is observed. This behavior is explained by the increase of the dehydrogenation of formic acid, which is formed as an intermediate, by the second catalyst B3 .
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