铀酰
电化学
法拉第效率
催化作用
格式化
水溶液
化学工程
材料科学
选择性
水溶液中的金属离子
吸附
纳米颗粒
无机化学
金属
铀
化学
电极
纳米技术
有机化学
冶金
物理化学
工程类
作者
Zhuanzhuan Zhai,Lifen Long,Xinpeng Che,Bailang Zhang,Ting Wang,Mingjie Li,Chaoxu Li
标识
DOI:10.1016/j.cej.2024.149402
摘要
Extraction of aqueous uranium element for practical applications has drawn growing attention due to its significance for both green energy acquirement and ecological environment remediation. Herein, the liquid metal droplets produced by a facile ultra-sonication process are found to be able to capture aqueous uranyl ions with a maximal adsorption capacity up to 237 mg g−1 (1483 mg cm−3), and further to reduce them into insoluble UO2 nanoparticles (2–5 nm in diameter). With the homogeneous immobilization of UO2 nanoparticles, the ultra-thin shell of liquid metal droplets exhibits a high catalytic activity towards electrochemical reductions e.g., CO2 reduction. The liquid metal core, when supporting on the electrodes, also offers the efficient electro-transporting pathway for electrochemical reaction. With a high formate selectivity, a faradaic efficiency ≥91.4 % and a generation rate as high as 988.9 mmol g−1h−1 of C1 products (i.e., CO and formate) are achieved in the CO2 reduction. Thus, this study may offer not only a unique platform of liquid metal nanodroplets for extracting uranium from water, but also a novel route of fabricating high-efficiency electrochemical catalysts for CO2 conversion.
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