材料科学
蜘蛛丝
纺纱
丝绸
复合材料
发光
纤维
光纤
纳米技术
光电子学
计算机科学
电信
作者
Kai Wen,Jiale Li,Guanghao Zhang,Meilin Wang,Guangkai Mei,Zhenzhen Zhang,Weiqiang Zhao,Wenjin Guo,Liqiang Zhou,Enzhao Liu,Yutian Zhu,Jie Bai,Meifang Zhu,Wei Wang,Zunfeng Liu,Xiang Zhou
标识
DOI:10.1002/adma.202314158
摘要
The development of functional surgical sutures with excellent mechanical properties, good fluorescence, and high cytocompatibility is highly required in the field of medical surgeries. Achieving fibers that simultaneously exhibit high mechanical robustness, good spinnability, and durable fluorescence emission has remained challenging up to now. Taking inspiration from the spinning process of spider silk and the luminescence mechanism of jellyfish, this work reports a luminous artificial spider silk prepared with the aim of balancing the fiber spinnability and mechanical robustness. This is realized by employing highly hydrated segments with aggregation-induced luminescence for enhancing the fiber spinnability and polyhydroxyl segments for increasing the fiber mechanical robustness. Twist insertion during fiber spinning improves the fiber strength, toughness, and fluorescence emission. Furthermore, coating the fiber with an additional polymer layer results in a "sheath-core" architecture with improved mechanical properties and capacity to withstand water. This work provides a new design strategy for performing luminescent and robust surgical sutures.
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