材料科学
矫顽力
铁磁性
成核
自旋电子学
单层
半导体
磁性半导体
凝聚态物理
饱和(图论)
磁化
基质(水族馆)
图层(电子)
反铁磁性
纳米技术
化学物理
光电子学
磁场
热力学
海洋学
物理
数学
组合数学
量子力学
地质学
作者
Xiangyi Wang,Liang Ma,Chuanlong Wang,Jiong Wang,Jun Guo,Rujun Tang,Juntong Zhu,Guifu Zou
标识
DOI:10.1002/adfm.202213295
摘要
The discovery of layered magnetic semiconductor materials has stimulated a search for the magnetic order of atomically thin-layered materials. However, layer-controlled growth is difficult because of the high nucleation barrier of the material surface during the few-layer formation of 2D materials. Herein, a seeding solution method is demonstrated that changes the nucleation mode of seed crystals on the substrate surface by precisely controlling the concentration of metal precursors and promoting the formation of cluster seed nuclei to ensure a sufficient source of metal for subsequent reactions. It is studied that the kinetic and thermodynamic synergy through temperature control is readily to grow VS2 with a tunable layer number. Monolayer VS2 exhibits strong ferromagnetic ordering with a saturation magnetization strength (Ms) of 37 emu per cc and a coercivity (Hc) of 135 Oe at 300 K. Notably, the ferromagnetism of VS2 has layer-dependent performance of the saturation magnetization and coercivity decreases with increasing number of layers. Monolayer VS2 exhibits typical semiconductor properties in Hall devices. This study broadens the chemical pathway for the tunable synthesis of 2D layered magnetic materials and provides the possibility for the construction of novel spintronic and magnetoelectronic devices.
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