色素敏化染料
材料科学
表面等离子共振
纳米颗粒
能量转换效率
图层(电子)
化学工程
电化学
等离子体子
煅烧
光电子学
纳米技术
光电效应
电极
电解质
化学
催化作用
工程类
物理化学
生物化学
作者
Fengjuan Miao,Fu-Chen Chu,Bingcheng Sun,Bairui Tao,Peng Zhang,Yu Zang,Paul K. Chu
标识
DOI:10.1016/j.jmrt.2022.09.060
摘要
A photoanode composed of Au/SnS/TiO2 sensitized by natural dye is designed and fabricated for dye-sensitized solar cells (DSSCs). A layer of spherical nano-TiO2 is prepared by calcination and a layer of nano-SnS is deposited on the TiO2 photoanode by the continuous ion layer adsorption reaction (SILAR). The Au nanoparticles are modified and sensitized with natural dye. The Au nanoparticles exhibit excellent localized surface plasmon resonance (LSPR) effects and enhanced the electron trapping ability. Owing to the smaller bandgap of SnS and optical activity in the infrared region, the electron mobility improves and electron recombination decreases. Electrochemical assessment reveals that the photoelectric characteristics of the DSSC based on Au/SnS/TiO2 are greatly improved after natural dye sensitization and compared with the TiO2 photoanode, the power conversion efficiency (PCE) of the DSSC improves by 105%.
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