Flexible Pressure Sensor Decorated with MXene and Reduced Graphene Oxide Composites for Motion Detection, Information Transmission, and Pressure Sensing Performance

Although fiber-based flexible piezoresistive pressure sensors have received extensive attention because of their simple fabrication and easy integration, the common practice of using a single material as the sensing layer often leads to unsatisfactory sensitivity and a limited sensing range. Herein, we exploit the combination of reduced graphene oxide (rGO) and two-dimensional transition-metal carbides and nitrides (MXene), use a polyester filament (PET) as the fiber matrix, and fabricate an MX/rGO PET-based flexible pressure sensor using the "dipping-drying" method. A systematic study is conducted concerning the effect of the dip-coating sequence and material combination on the sensor's resistance and sensitivity, which reveals that MX/rGO PET has the smallest resistance and the highest sensitivity (1.24 kPa-1). A series of tests are conducted to evaluate the pressure sensing characteristics of the MX/rGO PET-based pressure sensor, confirming its good linearity, fast response speed, low detection limit, and stable performance. In addition, the sensor has been successfully used to monitor various human joint activities and physiological signals such as breathing, demonstrating great application potential in the field of personal health care. To further enhance the practical utility, an APP has been designed to analyze and display the collected signals, and the constructed sensor network also provides an ingenious method for information encryption and transmission via pressure sensing. In all, the MX/rGO PET-based pressure sensor proposed in this work is expected to provide a competitive scheme for wearable flexible electronic devices in information transmission and human-computer interaction in the future.