Formation, Detection, and Function of Oxygen Vacancy in Metal Oxides for Solar Energy Conversion

材料科学 能量转换 化学物理 纳米技术 金属 空位缺陷 氧气 化学工程 热力学 化学 结晶学 冶金 物理 工程类 有机化学
作者
Zhiliang Wang,Rijia Lin,Yuning Huo,Hexing Li,Lianzhou Wang
出处
期刊:Advanced Functional Materials [Wiley]
卷期号:32 (7) 被引量:177
标识
DOI:10.1002/adfm.202109503
摘要

Abstract Oxygen vacancy (V O ) is one of the most common defects in metal oxides (MOs), which endow the MOs with many unique physiochemical properties. Even though V O engineering has been applied in photo(electro)catalysis, there are still significant challenges in the understanding of the formation, structure, and property of V O . The V O can be produced by treating MOs under low oxygen atmosphere or in vacuum ruled by the equilibrium of V O formation, while other types of defects can also be generated simultaneously. Identifying and distinguishing the formation and function of Vo remain highly challenging, thus the scrutiny of defect formation energy and structure of V O is significant in V O research. This review critically revisits the electronic property and structure changes of MOs upon the generation of Vo. It not only provides clues to detect V O , but also specifies the role of V O in a particular material system considering its drastic influence on light harvesting, conductivity, energy level, surface adsorption, and others. The review also presents a perspective on the future research directions toward rational control of the key aspects of Vo in MOs, namely its formation, characterization, and function, for solar energy conversion.
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