光降解
罗丹明B
盐酸四环素
光催化
三元运算
材料科学
核化学
催化作用
化学工程
化学
光化学
四环素
有机化学
生物化学
工程类
程序设计语言
抗生素
计算机科学
作者
Zhihong Wu,Lingfu Yang,Xiaofeng Yang,Yunqin Gao,Xinwei Li,Meidan Que,Ta‐I Yang,Zhikang Liu,Huiqi Zheng,Youguang Ma,Yanjun Li,Jin Chen
标识
DOI:10.1016/j.jallcom.2023.168734
摘要
The photodegradation of antibiotics and organic dyes in water in the current environment has attracted attention. However, its practical value in the river is poor because the efficient and recyclable photocatalysts are insufficient. Therefore, a novel ternary BiOBr/g-C3N4/Ti3C2Tx (BCT-x) hybrids were efficaciously prepared via the in-situ construction method for improving photodegradation of Tetracycline Hydrochloride (TC-HCl) and Rhodamine B (RhB) under Xenon lamp. The characterization results clarified that the combination of BiOBr and g-C3N4 could expand light absorption region. Meanwhile, the hybrids possessed accelerated carrier separation and migration ability due to the introduction of co-catalyst Ti3C2Tx with efficient electrical conductivity. The BCT-5 exhibited vintage photocatalytic activity for TC-HCl (97%, 60 min) and RhB (98%, 50 min). Photo-generated holes (h+) and superoxide radicals (•O2−) were the main active species. The Liquid Chromatography and Mass Spectrometry (LC-MS) analysis showed that TC-HCl could be photodegraded by BCT-5 into smaller molecular weight and non-toxic substances. A reasonable photocatalytic mechanism on BiOBr/g-C3N4/Ti3C2Tx was brought up. This study provides guidance for advancing the application of photocatalytic technology in water pollutant degradation.
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