斜发沸石
再生(生物学)
环境科学
自然资源经济学
化学
生物
经济
沸石
生物化学
细胞生物学
催化作用
作者
Bo Jiang,Bo Zhang,Xiaoge Duan,Yi Xing
标识
DOI:10.1007/s40789-023-00661-x
摘要
Abstract This study focuses on CO 2 capture by pressure swing adsorption (PSA), with modified clinoptilolite as the adsorbent. Natural clinoptilolite is modified by roasting, by acid pickling, by a combination of acid pickling and roasting, and by ion exchange. Modification by acid pickling–roasting and by ion exchange are found to give the highest CO 2 adsorption capacities, of 730 mL/g and 876.7 mL/g, respectively. It is found that regeneration of clinoptilolite by a combination of vacuum desorption and heating enables recovery of as much as 89% of its previous CO 2 adsorption capacity. To examine the CO 2 adsorption capacity of clinoptilolite when applied to mixed gas, a simulated coking exhaust containing 12% CO 2 and 4% O 2 is used, and it is found that ion exchange modified clinoptilolite achieves a CO 2 removal efficiency of 92.5%. A BET test reveals that acid pickling–roasting and Na + modification enhance the porosity of clinoptilolite, thereby improving its adsorption capacity. This work demonstrates the feasibility of applying modified clinoptilolite as an effective adsorbent for CO 2 capture, providing a promising tool for dealing with greenhouse gases.
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