Oxygen Evolution Reaction In article number 2307069, Zhisheng Wu, Zhi Fang, Qing Shi, and co-workers report a simple and fast strategy to promote self reconstruction of NiFe-layered double hydroxides and form highly active NiFeOOH centers. The trace Zn dopants have been introduced in advance, followed by leaching over the electrochemical activation process. The self-restructured NiFeOOH-VZn exhibits excellent catalytic activity and stability for the oxygen evolution reaction.