A novel reed‐leaves like aluminum‐doped manganese oxide presetting sodium‐ion constructed by coprecipitation method for high electrochemical performance sodium‐ion battery

International Journal of Energy ResearchVolume 46, Issue 10 p. 14570-14580 TECHNICAL NOTE A novel reed-leaves like aluminum-doped manganese oxide presetting sodium-ion constructed by coprecipitation method for high electrochemical performance sodium-ion battery Kedi Cai, Kedi Cai orcid.org/0000-0003-1309-1928 College of Chemistry and Materials Engineering, Bohai University, Jinzhou, China Liaoning Engineering Technology Research Center of Supercapacitor, Bohai University, Jinzhou, ChinaSearch for more papers by this authorXueqin Jing, Xueqin Jing College of Chemistry and Materials Engineering, Bohai University, Jinzhou, ChinaSearch for more papers by this authorYuting Zhang, Yuting Zhang College of Chemistry and Materials Engineering, Bohai University, Jinzhou, ChinaSearch for more papers by this authorLan Li, Lan Li Center for Experiment, Bohai University, Jinzhou, ChinaSearch for more papers by this authorXiaoshi Lang, Corresponding Author Xiaoshi Lang [email protected] orcid.org/0000-0001-5780-1261 College of Chemistry and Materials Engineering, Bohai University, Jinzhou, China Liaoning Engineering Technology Research Center of Supercapacitor, Bohai University, Jinzhou, China Correspondence Xiaoshi Lang, College of Chemistry and Materials Engineering, Bohai University, Jinzhou 121013, China. Email: [email protected]Search for more papers by this author Kedi Cai, Kedi Cai orcid.org/0000-0003-1309-1928 College of Chemistry and Materials Engineering, Bohai University, Jinzhou, China Liaoning Engineering Technology Research Center of Supercapacitor, Bohai University, Jinzhou, ChinaSearch for more papers by this authorXueqin Jing, Xueqin Jing College of Chemistry and Materials Engineering, Bohai University, Jinzhou, ChinaSearch for more papers by this authorYuting Zhang, Yuting Zhang College of Chemistry and Materials Engineering, Bohai University, Jinzhou, ChinaSearch for more papers by this authorLan Li, Lan Li Center for Experiment, Bohai University, Jinzhou, ChinaSearch for more papers by this authorXiaoshi Lang, Corresponding Author Xiaoshi Lang [email protected] orcid.org/0000-0001-5780-1261 College of Chemistry and Materials Engineering, Bohai University, Jinzhou, China Liaoning Engineering Technology Research Center of Supercapacitor, Bohai University, Jinzhou, China Correspondence Xiaoshi Lang, College of Chemistry and Materials Engineering, Bohai University, Jinzhou 121013, China. Email: [email protected]Search for more papers by this author First published: 14 May 2022 https://doi.org/10.1002/er.8090Citations: 2 Funding information: Science and Technology General Project of Liaoning Province Education Department, Grant/Award Numbers: LQ2020009, LZ2020002; Support Program of Distinguished Professor of Liaoning Province, Grant/Award Number: 071717002; Distinguished Professor of Liaoning Province; National Natural Science Foundation of China, Grant/Award Number: 22075030 Read the full textAboutPDF ToolsRequest permissionExport citationAdd to favoritesTrack citation ShareShare Give accessShare full text accessShare full-text accessPlease review our Terms and Conditions of Use and check box below to share full-text version of article.I have read and accept the Wiley Online Library Terms and Conditions of UseShareable LinkUse the link below to share a full-text version of this article with your friends and colleagues. Learn more.Copy URL Share a linkShare onEmailFacebookTwitterLinkedInRedditWechat Summary In this paper, Al-doped manganese oxide with presetting sodium-ion (NaxMnyAlzO2) is synthesized by a facile coprecipitation method and combines with Na3V2(PO4)3 cathode active materials for sodium-ion battery in order to optimize the electrochemical performances. During the coprecipitation, a stable NaxMnyAlzO2 polynary metal oxide with Mn and Al molar ratio to 3:1 shows a special micromorphology similar to that of reed leaves, which makes it have a more ideal electrochemical specific surface area and ample mass transfer channels for rapid sodium-ion insertion and desorption. Electrochemical test indicates that reed-leaves like NaxMnyAlzO2 polynary metal oxides as active material for sodium-ion capacitor exhibit a very excellent reversibility and low electrochemical (Rct = 434 Ω) and concentration polarization (DNa+ = 2.2728 × 10−11 cm2 s−1). Specific discharge capacity can achieve to 73.76 F g−1 at 100 mA g−1 current density corresponding to 368.8 m2 g−1 electrochemical specific surface area. After 200 cycles, the capacity retention rate can be maintained at 81.81%. In addition, reed-leaves like NaxMnyAlzO2 polynary metal oxide playing a good depolarization role combined with Na3V2(PO4)3 active materials in the mass ratio to 7:3 can bring about the most excellent electrochemical performances. CONFLICT OF INTEREST The authors declare no conflict of interest. Open Research DATA AVAILABILITY STATEMENT The data that support the findings of this study are available from the corresponding author upon reasonable request. REFERENCES 1Fedotov SS, Luchinin ND, Aksyonov DA, et al. Titanium-based potassium-ion battery positive electrode with extraordinarily high redox potential. Nat Commun. 2020; 11: 1484. 2Cen Z, Kubiak P. Lithium-ion battery SOC/SOH adaptive estimation via simplified single particle model. 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Citing Literature Volume46, Issue10August 2022Pages 14570-14580 ReferencesRelatedInformation