Direct Observation of Spin–Orbit Interaction of Light via Chiroptical Responses

The spin-orbit interaction of light is a fundamental manifestation of controlling its angular momenta with numerous applications in photonic spin Hall effects and chiral quantum optics. However, observation of an optical spin Hall effect, which is normally very weak with subwavelength displacements, needs quantum weak measurements or sophisticated metasurfaces. Here, we theoretically and experimentally demonstrate the spin-orbit interaction of light in the form of strong chiroptical responses by breaking the in-plane inversion symmetry of a dielectric substrate. The chiroptical signal is observed at the boundary of a microdisk illuminated by circularly polarized vortex beams at normal incidence. The generated chiroptical spectra are tunable for different photonic orbital angular momenta and microdisk diameters. Our findings, correlating photonic spin-orbit interaction with chiroptical responses, may provide a route for exploiting optical information processing, enantioselective sensing, and chiral metrology.