Yujia Li,Wangying Xu,Wenjun Liu,Shun Han,Peijiang Cao,Ming Fang,Deliang Zhu,Youming Lu
出处
期刊:ACS applied electronic materials [American Chemical Society] 日期:2019-08-14卷期号:1 (9): 1842-1851被引量:25
标识
DOI:10.1021/acsaelm.9b00377
摘要
We report the aqueous-solution-processed Ni-doped In2O3 (NixIn2–xO3, NiInO) thin-film transistors (TFTs) for the first time. The effect of Ni doping on In2O3 microstructure, oxygen defects, and the electron transport properties are investigated by extensive characterization techniques. Analyses indicate that the oxygen vacancies in NiInO are suppressed as the Ni-doping concentration increases, leading to a lower off-state current and a positive shift in threshold voltage. The optimized NiInO TFTs exhibit a high mobility of 17.71 cm2/(V s), on/off current ratio > 106, threshold voltage of 4.21 V, and superior bias stress stability. The success of Ni doping could be attributed to the small ion radius of Ni, large Lewis acid value, and strong Ni–O bond strength. Therefore, the fabricated NiInO TFT provides a bright path for the development of high-performance oxide TFTs.