光催化
材料科学
人工光合作用
太阳能燃料
半导体
可见光谱
光电子学
电化学
还原(数学)
氧化还原
分解水
纳米技术
光化学
金属
化学工程
电极
催化作用
化学
有机化学
冶金
工程类
物理化学
数学
几何学
标识
DOI:10.1002/adma.201808205
摘要
Abstract CO 2 reduction to carbon feedstocks using heterogeneous photocatalysts is an attractive means of addressing both climate change and the depletion of fossil fuels. Of particular importance is the development of a photosystem capable of functioning in response to visible light, which accounts for the majority of the solar spectrum, representing a kind of artificial photosynthesis. Hybrid systems comprising a metal complex and a semiconductor are promising because of the excellent electrochemical (and/or photocatalytic) activity of metal complexes during CO 2 reduction and the ability of semiconductors to efficiently oxidize water to molecular O 2 . Here, the development of hybrid photocatalysts and photoelectrodes for CO 2 reduction in combination with water oxidation is described.
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