Surface‐Plasmon‐Enhanced Photodriven CO2 Reduction Catalyzed by Metal–Organic‐Framework‐Derived Iron Nanoparticles Encapsulated by Ultrathin Carbon Layers

Advanced MaterialsVolume 28, Issue 19 p. 3703-3710 Communication Surface-Plasmon-Enhanced Photodriven CO2 Reduction Catalyzed by Metal–Organic-Framework-Derived Iron Nanoparticles Encapsulated by Ultrathin Carbon Layers Huabin Zhang, Huabin Zhang Environmental Remediation Materials Unitand International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS), 1-1 Namiki, Tsukuba, Ibaraki, 305-0044 JapanSearch for more papers by this authorTao Wang, Tao Wang Environmental Remediation Materials Unitand International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS), 1-1 Namiki, Tsukuba, Ibaraki, 305-0044 JapanSearch for more papers by this authorJunjie Wang, Junjie Wang Environmental Remediation Materials Unitand International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS), 1-1 Namiki, Tsukuba, Ibaraki, 305-0044 JapanSearch for more papers by this authorHuimin Liu, Huimin Liu Environmental Remediation Materials Unitand International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS), 1-1 Namiki, Tsukuba, Ibaraki, 305-0044 JapanSearch for more papers by this authorThang Duy Dao, Thang Duy Dao Environmental Remediation Materials Unitand International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS), 1-1 Namiki, Tsukuba, Ibaraki, 305-0044 Japan CREST, Japan Science and Technology Agency (JST), 4-1-18 Honcho, Kawaguchi, Saitama, 332-0012 JapanSearch for more papers by this authorMu Li, Mu Li Environmental Remediation Materials Unitand International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS), 1-1 Namiki, Tsukuba, Ibaraki, 305-0044 JapanSearch for more papers by this authorGuigao Liu, Guigao Liu Environmental Remediation Materials Unitand International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS), 1-1 Namiki, Tsukuba, Ibaraki, 305-0044 JapanSearch for more papers by this authorXianguang Meng, Xianguang Meng Environmental Remediation Materials Unitand International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS), 1-1 Namiki, Tsukuba, Ibaraki, 305-0044 JapanSearch for more papers by this authorKun Chang, Kun Chang Environmental Remediation Materials Unitand International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS), 1-1 Namiki, Tsukuba, Ibaraki, 305-0044 JapanSearch for more papers by this authorLi Shi, Li Shi Environmental Remediation Materials Unitand International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS), 1-1 Namiki, Tsukuba, Ibaraki, 305-0044 JapanSearch for more papers by this authorTadaaki Nagao, Tadaaki Nagao Environmental Remediation Materials Unitand International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS), 1-1 Namiki, Tsukuba, Ibaraki, 305-0044 Japan CREST, Japan Science and Technology Agency (JST), 4-1-18 Honcho, Kawaguchi, Saitama, 332-0012 JapanSearch for more papers by this authorJinhua Ye, Corresponding Author Jinhua Ye Environmental Remediation Materials Unitand International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS), 1-1 Namiki, Tsukuba, Ibaraki, 305-0044 Japan TU-NIMS Joint Research Center, School of Material Science and Engineering, Tianjin University, 92 Weijin Road, Nankai District, Tianjin, 300072 P. R. China Collaborative Innovation Center of Chemical Science and Engineering, (Tianjin), Tianjin, 300072 P. R. China Key Lab of Advanced Ceramics and Machining Technology, Ministry of Eduction, Tianjin, 300072 P. R. ChinaE-mail: jinhua.ye@nims.go.jpSearch for more papers by this author Huabin Zhang, Huabin Zhang Environmental Remediation Materials Unitand International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS), 1-1 Namiki, Tsukuba, Ibaraki, 305-0044 JapanSearch for more papers by this authorTao Wang, Tao Wang Environmental Remediation Materials Unitand International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS), 1-1 Namiki, Tsukuba, Ibaraki, 305-0044 JapanSearch for more papers by this authorJunjie Wang, Junjie Wang Environmental Remediation Materials Unitand International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS), 1-1 Namiki, Tsukuba, Ibaraki, 305-0044 JapanSearch for more papers by this authorHuimin Liu, Huimin Liu Environmental Remediation Materials Unitand International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS), 1-1 Namiki, Tsukuba, Ibaraki, 305-0044 JapanSearch for more papers by this authorThang Duy Dao, Thang Duy Dao Environmental Remediation Materials Unitand International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS), 1-1 Namiki, Tsukuba, Ibaraki, 305-0044 Japan CREST, Japan Science and Technology Agency (JST), 4-1-18 Honcho, Kawaguchi, Saitama, 332-0012 JapanSearch for more papers by this authorMu Li, Mu Li Environmental Remediation Materials Unitand International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS), 1-1 Namiki, Tsukuba, Ibaraki, 305-0044 JapanSearch for more papers by this authorGuigao Liu, Guigao Liu Environmental Remediation Materials Unitand International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS), 1-1 Namiki, Tsukuba, Ibaraki, 305-0044 JapanSearch for more papers by this authorXianguang Meng, Xianguang Meng Environmental Remediation Materials Unitand International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS), 1-1 Namiki, Tsukuba, Ibaraki, 305-0044 JapanSearch for more papers by this authorKun Chang, Kun Chang Environmental Remediation Materials Unitand International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS), 1-1 Namiki, Tsukuba, Ibaraki, 305-0044 JapanSearch for more papers by this authorLi Shi, Li Shi Environmental Remediation Materials Unitand International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS), 1-1 Namiki, Tsukuba, Ibaraki, 305-0044 JapanSearch for more papers by this authorTadaaki Nagao, Tadaaki Nagao Environmental Remediation Materials Unitand International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS), 1-1 Namiki, Tsukuba, Ibaraki, 305-0044 Japan CREST, Japan Science and Technology Agency (JST), 4-1-18 Honcho, Kawaguchi, Saitama, 332-0012 JapanSearch for more papers by this authorJinhua Ye, Corresponding Author Jinhua Ye Environmental Remediation Materials Unitand International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS), 1-1 Namiki, Tsukuba, Ibaraki, 305-0044 Japan TU-NIMS Joint Research Center, School of Material Science and Engineering, Tianjin University, 92 Weijin Road, Nankai District, Tianjin, 300072 P. R. China Collaborative Innovation Center of Chemical Science and Engineering, (Tianjin), Tianjin, 300072 P. R. China Key Lab of Advanced Ceramics and Machining Technology, Ministry of Eduction, Tianjin, 300072 P. R. ChinaE-mail: jinhua.ye@nims.go.jpSearch for more papers by this author First published: 22 March 2016 https://doi.org/10.1002/adma.201505187Citations: 250Read the full textAboutPDF ToolsRequest permissionExport citationAdd to favoritesTrack citation ShareShare Give accessShare full text accessShare full-text accessPlease review our Terms and Conditions of Use and check box below to share full-text version of article.I have read and accept the Wiley Online Library Terms and Conditions of UseShareable LinkUse the link below to share a full-text version of this article with your friends and colleagues. Learn more.Copy URL Share a linkShare onFacebookTwitterLinkedInRedditWechat Graphical Abstract Highly efficient utilization of solar light with an excellent reduction capacity is achieved for plasmonic Fe@C nanostructures. By carbon layer coating, the optimized catalyst exhibits enhanced selectivity and stability applied to the solar-driven reduction of CO2 into CO. The surface-plasmon effect of iron particles is proposed to excite CO2 molecules, and thereby facilitates the final reaction activity. Citing Literature Supporting Information As a service to our authors and readers, this journal provides supporting information supplied by the authors. Such materials are peer reviewed and may be re-organized for online delivery, but are not copy-edited or typeset. Technical support issues arising from supporting information (other than missing files) should be addressed to the authors. Filename Description adma201505187-sup-0001-S1.pdf3 MB Supplementary Please note: The publisher is not responsible for the content or functionality of any supporting information supplied by the authors. Any queries (other than missing content) should be directed to the corresponding author for the article. Volume28, Issue19May 18, 2016Pages 3703-3710 RelatedInformation