光催化
氮化碳
生物燃料
石墨氮化碳
材料科学
生物量(生态学)
环境友好型
纳米技术
生物炼制
催化作用
制氢
氢
碳纤维
环境科学
废物管理
化学
有机化学
复合数
生态学
工程类
复合材料
生物
作者
Jiliang Ma,Kangning Liu,Xiaopan Yang,Dongnv Jin,Yancong Li,Gaojie Jiao,Jinghui Zhou,Run‐Cang Sun
出处
期刊:Chemsuschem
[Wiley]
日期:2021-10-12
卷期号:14 (22): 4903-4922
被引量:41
标识
DOI:10.1002/cssc.202101173
摘要
Abstract Photoreforming of biomass into hydrogen, biofuels, and chemicals is highly desired, yet this field of research is still in its infancy. Developing an efficient, novel, and environmentally friendly photocatalyst is key to achieving these goals. To date, the nonmetallic and eco‐friendly material carbon nitride has found many uses in reactions such as water splitting, CO 2 reduction, N 2 fixation, and biorefinery, owing to its outstanding photocatalytic activity. However, a narrow light absorption range and fast charge recombination are often encountered in the pristine carbon nitride photocatalytic system, which resulted in unsatisfying photocatalytic activity. To improve the photocatalytic performance of pure carbon nitride in biomass reforming, modification is needed. In this Review, the design and preparation of functional carbon nitride, as well as its photocatalytic properties for the synthesis of hydrogen, biofuels, and chemicals through biomass reforming, are discussed alongside potential avenues for its future development.
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