Dimensionality-dependent type-II Weyl semimetal state in Mo0.25W0.75Te2

Weyl nodes and Fermi arcs in type-II Weyl semimetals (WSMs) have led to lots of exotic transport phenomena. Recently, ${\mathrm{Mo}}_{0.25}{\mathrm{W}}_{0.75}{\mathrm{Te}}_{2}$ has been established as a type-II WSM with Weyl points located near Fermi level, which offers an opportunity to study its intriguing band structure by electrical transport measurements. Here, by selecting a special sample with the thickness gradient across two- (2D) and three-dimensional (3D) regimes, we show strong evidence that ${\mathrm{Mo}}_{0.25}{\mathrm{W}}_{0.75}{\mathrm{Te}}_{2}$ is a type-II Weyl semimetal by observing the following two dimensionality-dependent transport features: (1) a chiral-anomaly-induced anisotropic magnetoconductivity enhancement, proportional to the square of in-plane magnetic field (${B}_{\mathrm{in}}^{2}$); and (2) an additional quantum oscillation with thickness-dependent phase shift. Our theoretical calculations show that the observed quantum oscillation originates from a Weyl-orbit-like scenario due to the unique band structure of ${\mathrm{Mo}}_{0.25}{\mathrm{W}}_{0.75}{\mathrm{Te}}_{2}$. The in situ dimensionality-tuned transport experiment offers an alternative strategy to search for type-II WSMs.