Core–Sheath Heterogenous Interlocked Stretchable Conductive Fiber Induced by Adhesive MXene Modulated Interfacial Soldering

Whereas high electrical conductivity and mechanical stretchability are both essentially required for flexible electronics, simultaneously achieving them remains a great challenge due to the "trade-off" effect. Herein, an ultrastretchable conductor with core-sheath heterogeneous interlocked structure was developed, induced by interfacial soldering silver nanowires (AgNWs) which gradually evolved into elastic conductive fiber. Adhesive polydopamine-functionalized MXene (PDM) was proposed as an interfacial solder to assemble AgNWs along fibers while induced strong cold-welding effect soldered them into superelastic interconnected network.