光催化
纳米颗粒
催化作用
材料科学
沉积(地质)
表面等离子共振
可见光谱
胶体金
等离子体子
光化学
光谱学
甲烷
吸收(声学)
降水
化学工程
辐照
纳米技术
化学
光电子学
有机化学
量子力学
沉积物
核物理学
复合材料
气象学
古生物学
工程类
物理
生物
作者
Laura Collado,Anna Reynal,Juan M. Coronado,David Serrano,James R. Durrant,Víctor A. de la Peña O’Shea
标识
DOI:10.1016/j.apcatb.2014.09.032
摘要
Various gold-supported TiO2 catalysts (0.5–3.0 wt.%) were prepared by a deposition–precipitation method, and their photocatalytic activity towards CO2 reduction was tested in the gas phase while using H2O as electron donor and UV and visible light as energy sources. CO and H2 are detected as major products in bare TiO2. However, the deposition of small Au nanoparticles (NPs) onto TiO2 was found to quantitatively enhance the reduction of CO2 mainly to methane and C2+ hydrocarbons. Transient absorption spectroscopy was used to correlate the improved CH4 production with an increased charge separation due to the electron transfer between the TiO2 and Au NPs. The amount of Au loaded onto TiO2 was optimized, with 1.0 wt.% showing the highest photocatalytic activity under UV light. Under visible irradiation, H2 and CH4 were identified as the main products, although showing significantly lower productions.
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