钙钛矿(结构)
材料科学
胶粘剂
压力(语言学)
导电体
各向异性
探测器
热的
复合材料
热膨胀
光电子学
结晶学
光学
化学
物理
热力学
哲学
语言学
图层(电子)
作者
Zhiqiang Liu,Haodi Wu,Haoming Yang,Zihao Song,Xinyuan Du,Xin He,Wuchen Xiang,Yunjing Shi,Jincong Pang,Ling Xu,Zhiping Zheng,Yao Zhang,Jiang Tang,Liduo Wang
出处
期刊:ACS energy letters
[American Chemical Society]
日期:2024-03-05
卷期号:9 (4): 1397-1404
标识
DOI:10.1021/acsenergylett.4c00195
摘要
Polycrystalline perovskite films offer promise for next-generation X-ray flat-panel detectors due to their ease of large-area fabrication. However, the perovskite–thin-film transistor (TFT) manufacturing mismatch causes defects (e.g., pores, fracture, and delamination), impacting device yield and dead pixel rates. We identify that thermal stress between the perovskite film and TFT array plays a pivotal role in causing these defects. We first propose the strategy of adding an anisotropic conductive adhesive as a stress buffer layer at the original interface. The Tresca stress at the interface was reduced from 113 to 58 MPa. The film fracture, pinhole, and delamination have been suppressed, and the device could even sustain a long-term vibration fatigue test. The assembled FPD exhibits 0.52 lp/pix spatial resolution and a 0.63% dead pixel rate, which outperform previous studies. This approach provides new insights and avenues for the fabrication of integrated perovskite–TFT devices with enhanced interface connectivity.
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