Modulating the Electrical Transport in Superconducting NbC Crystals by Fractal Morphology

材料科学 介观物理学 超导电性 分形 电阻率和电导率 凝聚态物理 超导相干长度 非平衡态热力学 纳米尺度 纳米技术 化学物理 热力学 数学 量子力学 物理 数学分析
作者
Yunqi Fu,Su Sun,Meng Hao,Qiang Wang,Zhibo Liu,Chuan Xu,Hui‐Ming Cheng,Wencai Ren,Ning Kang
出处
期刊:ACS Applied Materials & Interfaces [American Chemical Society]
卷期号:16 (44): 60865-60873
标识
DOI:10.1021/acsami.4c13602
摘要

The self-similar fractal morphology mediated by nonequilibrium processes is widely observed in low-dimensional materials grown by various techniques. Understanding how these fractal geometries affect the physical and chemical properties of materials and devices is crucial for both fundamental studies and various applications. In particular, the interplay between superconducting phase fluctuations and disorder can give rise to intriguing phenomena depending on the dimensionality. However, current experimental studies on low-dimensional superconductors are limited to two- and one-dimensional systems, leaving fractional dimensional systems largely unexplored. Here, we use chemical vapor deposition to successfully synthesize ultrathin NbC crystals with a well-defined fractal geometry at the nanoscale. By performing electrical transport measurements, we find that both the superconducting and normal-state properties are strongly affected in the fractal samples, where the intrinsic and geometric disorder is induced. In contrast to the 2D crystal, the fractal NbC crystals show a significant low-temperature resistive upturn before the onset of superconducting transition, which can be attributed to the disorder-enhanced electron–electron interaction effect. From transport data analysis, we demonstrate that the superconducting transition in NbC is correlated to the strength of disorder and the fractional dimensions, revealing that nanoscale fractal structures can significantly modify the electronic properties of low-dimensional superconductors. Our work paves the way for the explorations of mesoscopic transport and intriguing superconducting phenomena in fractional dimensions.
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