催化作用
纳米技术
电催化剂
介孔材料
材料科学
碳纤维
化学
电化学
电极
有机化学
复合材料
复合数
物理化学
作者
Zhenhui Liu,Yue Du,Pengfei Zhang,Zechao Zhuang,Dingsheng Wang
出处
期刊:Matter
[Elsevier]
日期:2021-10-01
卷期号:4 (10): 3161-3194
被引量:120
标识
DOI:10.1016/j.matt.2021.07.019
摘要
Rationally designing an appropriate support plays significant roles in catalysis through anchoring active sites firmly, enabling fast mass transport, and confining reaction fields. Recently, nitrogen-doped ordered mesoporous carbons (NOMCs) are emerging as an intriguing support due to well-defined ordered pore channels, unique confined microenvironment, and abundant N ligands, which create more possibilities of achieving catalytic orders and designing better catalysts. Here, we firstly cover the potentials of NOMCs in designing desirable catalysts with special emphasis on the characters of NOMCs toward catalysis. Then, various synthetic strategies for NOMCs are summarized, including (1) nanocasting, (2) solution collaborative self-assembly, (3) evaporation-induced self-assembly, and (4) solvent-free method. Next, we detail the catalytic applications of NOMCs-based metal-free, metal-nanoparticle, and single-atom catalysts across electrocatalysis and organic synthesis. Finally, we give a perspective for NOMCs about the current challenges and future opportunities confronted in their fundamental research and practical applications.
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