材料科学
纳米孔
钙钛矿(结构)
激光阈值
纳米激光器
纳米结构
成核
纳米技术
纳米尺度
光电子学
结晶
化学工程
波长
工程类
有机化学
化学
作者
Fengxian Zhou,Zhuocheng Chen,Zhiping Hu,Sihao Huang,Qian Li,Z. Zhan,Zhengzheng Liu,Zeyu Zhang,Jin He,Juan Du
标识
DOI:10.1002/adom.202300353
摘要
Abstract Perovskite micro/nanostructure with regular compact structure and high optical gain has provided a viable route toward the miniaturization of micro/nanolaser without an external cavity. Herein, a new process for the ultra‐rapid room‐temperature synthesis of perovskite micro/nanocubes with controllable size by combining surface‐induced crystallization with the perovskite solution route is described. At first, the perovskite precursors PbBr 2 are encapsulated into the nanoporous glass monolith and then react with CsBr solution on a glass surface, where nanoscopic pores facilitate heterogeneous nucleation significantly. The whole synthesis process of micro/nanocubes is ultra‐rapid and complete within 20 s. Based on the synthetic perovskite micro/nanocubes, low‐threshold upconversion lasing is successfully realized with a high‐quality factor of 2845, which further confirms the high quality and excellent optical performance of perovskite micro/nanocubes. This powerful solution route provides an ultra‐rapid and facile method for the synthesis of perovskite micro/nanostructure toward miniaturized optoelectronic devices.
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