快速重离子
辐照
材料科学
通量
薄膜
带隙
光电子学
辐射硬化
X射线光电子能谱
离子
辐射损伤
纳米技术
化学
物理
核物理学
核磁共振
有机化学
作者
Yongtao Yang,Yuanjun Tang,Fanyu Liu,Lei Wang,Fan Zhang,Tie-Jun Wang,Lei Shu,Zhenping Wu,Huiping Zhu,Bo Li,Danfeng Li
标识
DOI:10.1016/j.apsusc.2023.158583
摘要
The ultra-wide band gap (∼4.9 eV) and extremely large breakdown field strength (∼8 MV/cm) enable ε-Ga2O3 as an ideal materials candidate for high-performance power devices and solar-blind photodetectors. For the purpose of deep space applications explorations, comprehensive study of the effects of particle irradiation on the lattice stability and electronic properties of ε-Ga2O3 are of pivotal importance. In this work, leveraging a unique Ta radiation source, we interrogate the radiation hardness of ε-Ga2O3 thin films after 1907 MeV Ta swift heavy ion (SHI) irradiation. Detailed characterizations of the structural and optical properties show that the morphology and lattice structure are disrupted, with an increase of the band gap. Additionally, X-ray photoelectron spectroscopy experiments combining density functional theory calculations corroborate extrinsic flux-induced high concentration defects in the film, which lead to truncated photo-response performance of the device. However, even upon irradiation with a fluence of 5 × 1010 cm−2, the overall performance of the device remains robust and substantial. This outstanding radiation hardness of ε-Ga2O3 thin films rationalizes their potential usage for space applications.
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