光致发光
材料科学
量子产额
量子点
带隙
兴奋剂
荧光
石墨氮化碳
分析化学(期刊)
光电子学
可见光谱
波长
光化学
光学
光催化
化学
物理
有机化学
催化作用
作者
Jiang Wu,Siwei Yang,Jipeng Li,Yucheng Yang,Gang Wang,Xiuming Bu,Peng He,Jing Sun,Junhe Yang,Yuan Deng,Guqiao Ding,Xiaoming Xie
标识
DOI:10.1002/adom.201600570
摘要
The large band gap (2.7 eV) of graphite‐like carbon nitride (g‐C 3 N 4 ) enables the g‐C 3 N 4 quantum dots (g‐C 3 N 4 QDs) to show near ultraviolet‐blue photoluminescence. This study demonstrates the effective band gap control of g‐C 3 N 4 QDs by phosphorus doping for the first time. With the electronic injection process of lattice doped P, the band gap decreased observably. The emission wavelength of phosphorus doped g‐C 3 N 4 QDs (P‐g‐C 3 N 4 QDs) can be tuned in whole visible light range (385–762 nm) by changing the doping concentration. Due to the direct band gap of these P‐g‐C 3 N 4 QDs, the quantum yield is higher than 0.90. The authors also show the application value of these P‐g‐C 3 N 4 QDs in both in vitro and in vivo fluorescent bio‐imaging.
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