Innovations in metal-organic frameworks (MOFs): Pioneering adsorption approaches for persistent organic pollutant (POP) removal

吸附 环境修复 污染物 金属有机骨架 环境科学 环境污染 纳米技术 生化工程 材料科学 化学 污染 工程类 环境保护 有机化学 生态学 生物
作者
Deepali Marghade,Sagar Shelare,Chander Prakash,Manzoore Elahi M. Soudagar,T. M. Yunus Khan,M.A. Kalam
出处
期刊:Environmental Research [Elsevier]
卷期号:258: 119404-119404 被引量:7
标识
DOI:10.1016/j.envres.2024.119404
摘要

Adsorption is a promising way to remove persistent organic pollutants (POPs), a major environmental issue. With their high porosity and vast surface areas, MOFs are suited for POP removal due to their excellent adsorption capabilities. This review addresses the intricate principles of MOF-mediated adsorption and helps to future attempts to mitigate organic water pollution. This review examines the complicated concepts of MOF-mediated adsorption, including MOF synthesis methodologies, adsorption mechanisms, and material tunability and adaptability. MOFs' ability to adsorb POPs via electrostatic forces, acid-base interactions, hydrogen bonds, and pi-pi interactions is elaborated. This review demonstrates its versatility in eliminating many types of contaminants. Functionalizing, adding metal nanoparticles, or changing MOFs after they are created can improve their performance and remove contaminants. This paper also discusses MOF-based pollutant removal issues and future prospects, including adsorption capacity, selectivity, scale-up for practical application, stability, and recovery. These obstacles can be overcome by rationally designing MOFs, developing composite materials, and improving material production and characterization. Overall, MOF technology research and innovation hold considerable promise for environmental pollution solutions and sustainable remediation. Desorption and regeneration in MOFs are also included in the review, along with methods for improving pollutant removal efficiency and sustainability. Case studies of effective MOF regeneration and scaling up for practical deployment are discussed, along with future ideas for addressing these hurdles.
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