Quasi-two dimensional Ruddlesden-Popper halide perovskites for laser applications

Abstract Quasi-two-dimensional (2D) Ruddlesden–Popper (RP) halide perovskites, as a kind of emerged two-dimensional layered materials, have recently achieved great attentions in lasing materials field owing to their large exciton binding energy, high emission yield, large optical gain, and wide-range tuning of optical bandgap. This review will introduce research progresses of RP halide perovskites for lasing applications in aspects of materials, photophysics, and devices with emphasis on emission and lasing properties tailored by the molecular composition and interface. The materials, structures and fabrications are introduced in the first part. Next, the optical transitions and amplified spontaneous emission properties are discussed from the aspects of electronic structure, exciton, gain dynamics, and interface tailoring. Then, the research progresses on lasing devices are summarized and several types of lasers including VCSEL, DFB lasers, microlasers, random lasers, plasmonic lasers, and polariton lasers are discussed. At last, the challenges and perspectives would be provided.