气凝胶
海水淡化
材料科学
废水
复合数
生物量(生态学)
蒸发器
太阳能淡化
化学工程
纳米技术
环境科学
环境工程
复合材料
化学
膜
生态学
工程类
机械工程
生物化学
热交换器
生物
作者
Shilin Chen,Dafeng Zheng,Qiulan Cen,Chang Geun Yoo,Lei Zhong,Dongjie Yang,Xueqing Qiu
出处
期刊:Small
[Wiley]
日期:2024-04-24
被引量:3
标识
DOI:10.1002/smll.202400603
摘要
Abstract Solar‐driven interfacial evaporation is recognized as a sustainable and effective strategy for desalination to mitigate the freshwater scarcity issue. Nevertheless, the challenges of oil contamination, salt accumulation, and poor long‐term stability of the solar desalination process limit its applications. Herein, a 3D biomass‐based multifunctional solar aerogel evaporator is developed for water production with fabricated chitosan/lignin (CSL) aerogel as the skeleton, encapsulated with carbonized lignin (CL) particles and Ti 3 C 2 Ti X (MXene) nanosheets as light‐absorbing materials. Benefitting from its super‐hydrophilic wettability, interconnected macropore structure, and high broadband light absorption (ca. 95.50%), the prepared CSL‐C@MXene‐20 mg evaporator exhibited a high and stable water evaporation flux of 2.351 kg m −2 h −1 with an energy conversion efficiency of 88.22% under 1 Sun (1 kW m −2 ) illumination. The CSL‐C@MXene‐20 mg evaporator performed excellent salt tolerance and long‐term solar vapor generation in a 3.5 wt.% NaCl solution. Also, its super‐hydrophilicity and oleophobicity resulted in superior salt resistance and anti‐fouling performance in high salinity brine (20 wt.% NaCl) and oily wastewater. This work offers new insight into the manufacture of porous and eco‐friendly biomass‐based photothermal aerogels for advanced solar‐powered seawater desalination and wastewater purification.
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