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Advances in hybrid strategies for enhanced photocatalytic water splitting: Bridging conventional and emerging methods

桥接(联网) 光催化 分解水 材料科学 纳米技术 计算机科学 工艺工程 化学 工程类 催化作用 计算机网络 生物化学
作者
Sandeep Kumar Lakhera,K. Priyanga Kangeyan,Crescentia Yazhini S,Shiny Golda A,Bernaurdshaw Neppolian
出处
期刊:Applied physics reviews [American Institute of Physics]
卷期号:11 (4)
标识
DOI:10.1063/5.0218539
摘要

Significant efforts have been dedicated to hydrogen production through photocatalytic water splitting (PWS) over the past five decades. However, achieving commercially viable solar-to-hydrogen conversion efficiency in PWS systems remains elusive. These systems face intrinsic and extrinsic challenges, such as inadequate light absorption, insufficient charge separation, limited redox active sites, low surface area, and scalability issues in practical designs. To address these issues, conventional strategies including heterojunction engineering, plasmonics, hybridization, lattice defects, sensitization, and upconversion processes have been extensively employed. More recently, innovative hybrid strategies like photonic crystal-assisted and polarization field-assisted PWS have emerged, which improve light absorption and charge separation by harnessing the slow photon effect, multiple light scattering, and the piezoelectric, pyroelectric, and ferroelectric properties of materials. This review article aims to provide a comprehensive examination and summary of these new synergistic hybrid approaches, integrating plasmonic effects, upconversion processes, and photonic crystal photocatalysis. It also explores the role of temperature in suppressing exciton recombination during photothermic photocatalysis. This article also highlights emerging strategies such as the effects of magnetic fields, periodic illumination, many-body large-hole polaron, and anapole excitations, which hold significant potential to advance PWS technology and facilitate renewable hydrogen generation.
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