Carbon-Based Piezoresistive Polymer Nanocomposites by Extrusion Additive Manufacturing: Process, Material Design, and Current Progress

Advancement in additive manufacturing (AM) allows the production of nanocomposites with complex and custom geometries not typically allowable with conventional manufacturing techniques. The benefits of AM have led to recent interest in producing multifunctional materials capable of being printed with current AM technologies. In this article, piezoresistive composites realized by AM and the matrices and fillers utilized to make such devices are introduced and discussed. Carbon-based nanoparticles (Carbon Nanotubes, Graphene/Graphite, and Carbon Black) are often the filler choice of most researchers and are heavily discussed throughout this review in combination with extrusion AM methods. Piezoresistive applications such as physiological and wearable sensors, structural health monitoring, and soft robotics are presented with an emphasis on material and AM selection to meet the demands of such applications.