Tunable Bandgap Energy and Promotion of H2O2 Oxidation for Overall Water Splitting from Carbon Nitride Nanowire Bundles

Advanced Energy MaterialsVolume 6, Issue 11 1502352 Communication Tunable Bandgap Energy and Promotion of H2O2 Oxidation for Overall Water Splitting from Carbon Nitride Nanowire Bundles Kan Zhang, Kan Zhang Department of Chemical and Biomolecular Engineering, Yonsei University, 50 Yonsei-ro, Seodaemun-gu, Seoul, 120-749 Republic of KoreaSearch for more papers by this authorLuyang Wang, Luyang Wang National Creative Research Initiative, Center for Smart Molecular Memory, Department of Chemistry, Energy Science and SAINT, Sungkyunkwan University, 2066 Seoburo, Jangan-Gu, Suwon, Gyeonggi-Do, 440-746 Republic of Korea [+]Present address: Department of Applied Biology and Chemical Technology, The Hong Kong Polytechnic University, Kowloon, Hong Kong, P. R. ChinaSearch for more papers by this authorXiaowei Sheng, Xiaowei Sheng Department of Physics, Anhui Normal University, Anhui, Wuhu, 241000 P. R. ChinaSearch for more papers by this authorMing Ma, Ming Ma Department of Chemical and Biomolecular Engineering, Yonsei University, 50 Yonsei-ro, Seodaemun-gu, Seoul, 120-749 Republic of Korea SKKU Advanced Institute of Nanotechnology, Sungkyunkwan University, Suwon, 440-746 Republic of KoreaSearch for more papers by this authorMyung Sun Jung, Myung Sun Jung Department of Chemical and Biomolecular Engineering, Yonsei University, 50 Yonsei-ro, Seodaemun-gu, Seoul, 120-749 Republic of KoreaSearch for more papers by this authorWanjung Kim, Wanjung Kim Department of Chemical and Biomolecular Engineering, Yonsei University, 50 Yonsei-ro, Seodaemun-gu, Seoul, 120-749 Republic of Korea School of Chemical Engineering, Sungkyunkwan University, Suwon, 440-746 Republic of KoreaSearch for more papers by this authorHyoyoung Lee, Hyoyoung Lee National Creative Research Initiative, Center for Smart Molecular Memory, Department of Chemistry, Energy Science and SAINT, Sungkyunkwan University, 2066 Seoburo, Jangan-Gu, Suwon, Gyeonggi-Do, 440-746 Republic of KoreaSearch for more papers by this authorJong Hyeok Park, Corresponding Author Jong Hyeok Park Department of Chemical and Biomolecular Engineering, Yonsei University, 50 Yonsei-ro, Seodaemun-gu, Seoul, 120-749 Republic of KoreaE-mail: lutts@yonsei.ac.krSearch for more papers by this author Kan Zhang, Kan Zhang Department of Chemical and Biomolecular Engineering, Yonsei University, 50 Yonsei-ro, Seodaemun-gu, Seoul, 120-749 Republic of KoreaSearch for more papers by this authorLuyang Wang, Luyang Wang National Creative Research Initiative, Center for Smart Molecular Memory, Department of Chemistry, Energy Science and SAINT, Sungkyunkwan University, 2066 Seoburo, Jangan-Gu, Suwon, Gyeonggi-Do, 440-746 Republic of Korea [+]Present address: Department of Applied Biology and Chemical Technology, The Hong Kong Polytechnic University, Kowloon, Hong Kong, P. R. ChinaSearch for more papers by this authorXiaowei Sheng, Xiaowei Sheng Department of Physics, Anhui Normal University, Anhui, Wuhu, 241000 P. R. ChinaSearch for more papers by this authorMing Ma, Ming Ma Department of Chemical and Biomolecular Engineering, Yonsei University, 50 Yonsei-ro, Seodaemun-gu, Seoul, 120-749 Republic of Korea SKKU Advanced Institute of Nanotechnology, Sungkyunkwan University, Suwon, 440-746 Republic of KoreaSearch for more papers by this authorMyung Sun Jung, Myung Sun Jung Department of Chemical and Biomolecular Engineering, Yonsei University, 50 Yonsei-ro, Seodaemun-gu, Seoul, 120-749 Republic of KoreaSearch for more papers by this authorWanjung Kim, Wanjung Kim Department of Chemical and Biomolecular Engineering, Yonsei University, 50 Yonsei-ro, Seodaemun-gu, Seoul, 120-749 Republic of Korea School of Chemical Engineering, Sungkyunkwan University, Suwon, 440-746 Republic of KoreaSearch for more papers by this authorHyoyoung Lee, Hyoyoung Lee National Creative Research Initiative, Center for Smart Molecular Memory, Department of Chemistry, Energy Science and SAINT, Sungkyunkwan University, 2066 Seoburo, Jangan-Gu, Suwon, Gyeonggi-Do, 440-746 Republic of KoreaSearch for more papers by this authorJong Hyeok Park, Corresponding Author Jong Hyeok Park Department of Chemical and Biomolecular Engineering, Yonsei University, 50 Yonsei-ro, Seodaemun-gu, Seoul, 120-749 Republic of KoreaE-mail: lutts@yonsei.ac.krSearch for more papers by this author First published: 29 March 2016 https://doi.org/10.1002/aenm.201502352Citations: 70 Read the full textAboutPDF ToolsRequest permissionExport citationAdd to favoritesTrack citation ShareShare Give accessShare full text accessShare full-text accessPlease review our Terms and Conditions of Use and check box below to share full-text version of article.I have read and accept the Wiley Online Library Terms and Conditions of UseShareable LinkUse the link below to share a full-text version of this article with your friends and colleagues. Learn more.Copy URL Share a linkShare onFacebookTwitterLinkedInRedditWechat Graphical Abstract A stepwise four-electron reaction significantly alleviates the thermodynamics reaction barrier for overall water splitting. Regenerated 1D carbon nitride nanowire bundles from tailoring and reassembly of 2D g-C3N4 produce novel physicochemical and optoelectronic properties, which well realize the stepwise four-electron reaction along with a quantum efficiency of 5.2‰ at 420 nm. Citing Literature Supporting Information As a service to our authors and readers, this journal provides supporting information supplied by the authors. Such materials are peer reviewed and may be re-organized for online delivery, but are not copy-edited or typeset. Technical support issues arising from supporting information (other than missing files) should be addressed to the authors. Filename Description aenm201502352-sup-0001-S1.pdf1 MB Supplementary Please note: The publisher is not responsible for the content or functionality of any supporting information supplied by the authors. Any queries (other than missing content) should be directed to the corresponding author for the article. Volume6, Issue11June 8, 20161502352 RelatedInformation