Liquid crystal monomers in soils near the e-waste recycling site and liquid crystal display manufacturer: Exponential decrease with distance

单体 土壤水分 液晶 指数函数 液晶显示器 材料科学 环境科学 废物管理 工程类 光电子学 土壤科学 聚合物 复合材料 数学 数学分析
作者
Jiong-Feng Xie,Gong‐Ping Wei,Lixi Zeng,Liang‐Ying Liu
出处
期刊:Science of The Total Environment [Elsevier]
卷期号:909: 168428-168428 被引量:3
标识
DOI:10.1016/j.scitotenv.2023.168428
摘要

Liquid crystal monomers (LCMs) have been recognized as contaminants of emerging concerns. E-waste recycling sites and liquid crystal displays (LCDs) manufacturers are supposed to be critical sources. However, information regarding LCM contaminations in soils surrounding these sites are currently unavailable. In this study, soil samples were collected from two distinct areas in South China: e-waste recycling area (n = 36) and LCD manufacturer (n = 41), and 60 target LCMs (including 13 biphenyl and analogs (BAs), 10 cyanobiphenyl and analogs (CBAs), and 37 fluorinated biphenyl and analogs (FBAs)) were determined. The concentrations of LCMs in the soils from near the e-waste recycling area (0.32–18 ng/g, average: 4.2 ng/g) were higher than those surrounding the LCD manufacturer (ND – 7.2 ng/g, average: 1.5 ng/g). The compositional profiles of LCMs in soil samples from these two typical point sources were considerably different. The concentrations of FBAs exponentially decreased with distance from the e-waste recycling park, by >90 % within 2 km. The levels of BAs exhibited a similar exponential decrease with distance from the LCD manufacturer. The inventories of LCMs were estimated to be 21.0 kg in the e-waste recycling area and 10.8 kg in the LCD manufacturer area. Remarkably, the inventory of LCMs in soils from e-waste recycling area was one order of magnitude larger than that of hexabromocyclododecanes (HBCDs) in the same region, and 0.2 to 20 times the annual global emissions of LCMs from discarded LCD panels. More studies are required to elucidate the environmental occurrence, behavior, and fate of LCMs in multimedia environment surrounding typical point sources.
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