Two-Dimensional Carbon Graphdiyne: Advances in Fundamental and Application Research

纳米技术 碳纤维 材料科学 复合数 复合材料
作者
Xuchen Zheng,Siao Chen,Jinze Li,Han Wu,Chao Zhang,Danyan Zhang,Xi Chen,Yang Gao,Feng He,Lan Hui,Huibiao Liu,Tonggang Jiu,Ning Wang,Guoxing Li,Jialiang Xu,Yurui Xue,Changshui Huang,Chunying Chen,Yanbing Guo,Tong‐Bu Lu
出处
期刊:ACS Nano [American Chemical Society]
卷期号:17 (15): 14309-14346 被引量:135
标识
DOI:10.1021/acsnano.3c03849
摘要

Graphdiyne (GDY), a rising star of carbon allotropes, features a two-dimensional all-carbon network with the cohybridization of sp and sp2 carbon atoms and represents a trend and research direction in the development of carbon materials. The sp/sp2-hybridized structure of GDY endows it with numerous advantages and advancements in controlled growth, assembly, and performance tuning, and many studies have shown that GDY has been a key material for innovation and development in the fields of catalysis, energy, photoelectric conversion, mode conversion and transformation of electronic devices, detectors, life sciences, etc. In the past ten years, the fundamental scientific issues related to GDY have been understood, showing differences from traditional carbon materials in controlled growth, chemical and physical properties and mechanisms, and attracting extensive attention from many scientists. GDY has gradually developed into one of the frontiers of chemistry and materials science, and has entered the rapid development period, producing large numbers of fundamental and applied research achievements in the fundamental and applied research of carbon materials. For the exploration of frontier scientific concepts and phenomena in carbon science research, there is great potential to promote progress in the fields of energy, catalysis, intelligent information, optoelectronics, and life sciences. In this review, the growth, self-assembly method, aggregation structure, chemical modification, and doping of GDY are shown, and the theoretical calculation and simulation and fundamental properties of GDY are also fully introduced. In particular, the applications of GDY and its formed aggregates in catalysis, energy storage, photoelectronic, biomedicine, environmental science, life science, detectors, and material separation are introduced.
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