分解水
混合动力系统
材料科学
半导体
能量转换
催化作用
接口(物质)
纳米技术
化学物理
光电子学
光催化
计算机科学
化学
物理
毛细管作用
毛细管数
复合材料
机器学习
热力学
生物化学
作者
Fujun Niu,Degao Wang,Fei Li,Yanming Liu,Shaohua Shen,Thomas J. Meyer
标识
DOI:10.1002/aenm.201900399
摘要
Photoelectrochemical (PEC) water splitting has attracted increasing attention due to its potential to mitigate energy and environmental issues. Hybrid PEC systems containing semiconductor photosensitizers and molecular catalysts are reported to be highly active and stable for water splitting with great potential for facilitating clean fuels production. In this review, following a showcasing of the fundamental details of hybrid PEC systems for water splitting, semiconductor/molecular catalyst interface designs are highlighted, with a focus on interfacial physicochemical interactions and binding, and interfacial energetics and dynamics for efficient charge transfer. Recent advances in hybrid system assemblies for PEC water splitting are also briefly introduced. Finally, future challenges and directions in the field of hybrid PEC water splitting for solar energy conversion are reviewed. The current review provides state‐of‐the‐art strategies for optimized interface design for creating highly active and stable PEC water splitting assemblies.
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