Magnetic Helicity in a Chiral‐Polar Magnet Ni2InSbO6

The class of chiral‐polar magnets has recently captured significant interest in scientific study due to their intriguing physical phenomena. Among all the chiral‐polar magnets, Ni 2 InSbO 6 stands out because of its unique attributes, such as the emergence of the topological chiral soliton lattice in the presence of an external magnetic field perpendicular to the chiral‐polar axis. However, the magnetic structure of Ni 2 InSbO 6 at zero field has not been well understood yet. This work presents an analysis including polarized optical microscopy and polarized neutron diffraction on a carefully chosen Ni 2 InSbO 6 crystal. Results confirm the predominance of a single chiral‐polar domain within the crystal and indicate the likelihood of cycloidal magnetic ordering under zero magnetic field, alongside the observation of net magnetic helicity. The existence of both a dominant chiral‐polar domain and a dominant cycloidal magnetic domain within Ni 2 InSbO 6 provides an excellent platform for further exploration of its unconventional physical attributes.